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Sakai, Hironori; Tokunaga, Yo; Kambe, Shinsaku; Zhu, J.-X.*; Ronning, F.*; Thompson, J. D.*; Kotegawa, Hisashi*; To, Hideki*; Suzuki, Kohei*; Oshima, Yoshiki*; et al.
Physical Review B, 106(23), p.235152_1 - 235152_8, 2022/12
Times Cited Count:0 Percentile:0(Materials Science, Multidisciplinary)We investigate the electronic state of Ni-substituted CeCoNiIn by nuclear quadrupole and magnetic resonance (NQR/NMR) techniques. The heavy fermion superconductivity below K for is suppressed by Ni substitutions, and reaches zero for . The In NQR spectra for and 0.25 can be explained by simulating the electrical field gradient that is calculated for a virtual supercell with density functional theory. The spin-lattice relaxation rate indicates that Ni substitution weakens antiferromagnetic correlations that are not localized near the substituent but instead are uniform in space. The temperature () dependence of for shows a maximum around K and decreases toward almost zero when temperature is further reduced as if a gap might be opening in the magnetic excitation spectrum; however, the magnetic specific heat and the static magnetic susceptibility evolve smoothly through with a dependence. The peculiar T dependence of and non-Fermi-liquid specific heat and susceptibility can be interpreted in a unified way by assuming nested antiferromagnetic spin fluctuations in a quasi-two-dimensional electronic system.
Yamada, Takashi*; Asai, Masato; Yonezawa, Chushiro*; Kakita, Kazutoshi*; Hirai, Shoji*
Radioisotopes, 69(9), p.287 - 297, 2020/09
We have confirmed that the commercially available Japanese "standard" gamma-ray analysis programs do not consider the effect of sample volume in calculating true coincidence summing (TCS) corrections, which results in underestimation of Cs radioactivity in cylindrical volume samples. In this work, we have developed and examined a practical TCS correction method for general Ge detectors which consider the effect of sample volume properly, and have confirmed that this method can reduce the Cs radioactivity underestimation to less than 1%.
Sanada, Yukihisa; Ochi, Kotaro; Ishizaki, Azusa
JAEA-Research 2020-006, 60 Pages, 2020/07
At the accident of nuclear facilities, a prediction of the behavior of released radioactive plume is indispensable to make a decision on a refuge plan of inhabitants. Currently, prediction system which is based on atmospheric dispersion simulation has been implemented as a tool of the atomic energy disaster prevention. However, the direct measurement method of the radioactive plume has not existed. In this study, some component technologies were developed for the establishment of direct measurement methods of radioactive plume using unmanned aerial vehicle whose technological innovation is remarkable. In addition, the spray test using mock aerosol was conducted to obtaining the deposition rate to the airplane body. The algorism of making a flight plan was developed based on a prediction model of the radioactive plume. This report summarized the outcome of the last year of the three-year plan.
Sanada, Yukihisa; Nishizawa, Yukiyasu*; Ochi, Kotaro; Yuki, Yoichi*; Ishizaki, Azusa; Osada, Naoyuki*
JAEA-Research 2018-009, 48 Pages, 2019/01
At the accident of nuclear facilities, a prediction of the behavior of released radioactive plume is indispensable to make a decision on a refuge plan of inhabitants. Currently, prediction system which is based on atmospheric dispersion simulation has been implemented as a tool of the atomic energy disaster prevention. However, the direct measurement method of the radioactive plume has not existed. In this study, some component technologies were developed for the establishment of direct measurement methods of radioactive plume using unmanned aerial vehicle whose technological innovation is remarkable. In addition, the spray test using mock aerosol was conducted to obtaining the deposition rate to the airplane body. The algorism of making a flight plan was developed based on a prediction model of the radioactive plume. This report summarized the outcome of the second year of the three-year plan.
Sakai, Hironori; Ronning, F.*; Hattori, Takanori; Tokunaga, Yo; Kambe, Shinsaku; Zhu, J.-X.*; Wakeham, N.*; Yasuoka, Hiroshi; Bauer, E. D.*; Thompson, J. D.*
Journal of Physics; Conference Series, 807(3), p.032001_1 - 032001_6, 2017/04
Times Cited Count:3 Percentile:68.62(Physics, Condensed Matter)We have used nuclear quadrupole resonance (NQR) to probe microscopically the response of a prototypical quantum critical metal CeCoIn to substitutions of small amounts of Cd for In. Approximately half of the Cd substituents induce local Ce moments in their close proximity, as observed by site-dependent longitudinal nuclear spin relaxation rates . To reaffirm that localized moments are induced around the Cd substituents, we find a Gaussian spin-echo decay rate of transverse nuclear spin relaxation. Further, for the NQR subpeak is found to be proportional to temperatures, again indicating local moments fluctuations around the Cd substituents, while that for the NQR main peak shows a -dependence. The latter temperature dependence is close to 0.75 in pure CeCoIn and indicates that the bulk electronic state is located close to a two dimensional quantum critical instability.
Van Beveren, C.*; Andreyev, A. N.; Barzakh, A. E.*; Cocolios, T. E.*; de Groote, R. P.*; Fedorov, D.*; Fedosseev, V. N.*; Ferrer, R.*; Ghys, L.*; Huyse, M.*; et al.
Journal of Physics G; Nuclear and Particle Physics, 43(2), p.025102_1 - 025102_22, 2016/02
Times Cited Count:11 Percentile:63.13(Physics, Nuclear)Asai, Masato; Heberger, F. P.*; Lopez-Martens, A.*
Nuclear Physics A, 944, p.308 - 332, 2015/12
Times Cited Count:54 Percentile:95.68(Physics, Nuclear)Nuclear structure of Z = 100-109 nuclei studied through -decay spectroscopy have been reviewed. Experimental techniques and methods concerning separation techniques, summing effects in spectra, and the use of digital electronics for -decay spectroscopy have been described in detail. The presentation of the experimental results and the physics discussion were focused on nuclear structure systematics in even-Z nuclei along the N = 151, 153, and 155 isotonic lines, where most progress has been achieved in the last 10 years.
Hosoma, Takashi
JAEA-Research 2015-009, 162 Pages, 2015/08
Neutron coincidence counting assay systems have been developed in the last two decades. Objects would extend to high-mass uranium-plutonium dioxide containing other spontaneous fission nuclei, so essentials of neutron multiplicity counting were reconsidered and expanded: (a) Formulae of multiplicity distribution were algebraically derived up to septuplet using a probability generating function; (b) Leakage multiplication was evaluated not by Monte Carlo method but by an average length from an arbitrary point inside a sample to an arbitrary point on its surface and a probability of induced fission within the length; (c) Mechanism of coincidence counting was associated with a couple of different time axes in Poisson process, and consequently a pair of close-to-coincident neutrons from the process was derived. For the formulae, new expressions using combination were wrote down. For spectrum and mean free path, actually treated uranium-plutonium dioxide was selected as an example.
Kaji, Daiya*; Morimoto, Koji*; Wakabayashi, Yasuo*; Takeyama, Mirei*; Asai, Masato
JPS Conference Proceedings (Internet), 6, p.030106_1 - 030106_4, 2015/06
A Si-Ge detector array was newly installed at the focal plane of the gas-filled recoil ion separator GARIS to perform - (X-rays) spectroscopy for superheavy nuclei. The performance of the array was tested using the Pb(Ca,2n)No and Pb(Ca,xn)No [x=1,2,3] reactions. rays originating from the decay of No and No were clearly observed in prompt coincidence with the particles.
Haraga, Tomoko; Kameo, Yutaka; Hoshi, Akiko; Yonezawa, Chushiro*; Nakashima, Mikio
JAERI-Tech 2005-050, 35 Pages, 2005/09
Non-destructive -ray spectrometry has been examined as a simple and rapid radioactivity measurement technique for the solidified products prepared by plasma melting for low level radioactive miscellaneous wastes generated from nuclear facilities. The Compton background resulting from the coexisting radionuclides pose a problem in the usual -ray spectrometry which uses only a Ge detector. In order to reduce the background count and to measure the interested nuclide selectively, the coincidence and the anti-coincidence -ray spectrometry using the Ge-BGO detector system were examined. As a result of applying the anti-coincidence -ray spectrometry to a single -ray emitter Cs and the coincidence -ray spectrometry to multiple -ray emitter Eu under existence of Co, the detection limits of Cs and Eu in the sample, which contained Co, were reduced by a factor of about 6 and 1.5, respectively. It was confirmed that the present methods are useful for the -activity measurement of solidified products.
Sakasai, Kaoru; Katagiri, Masaki; Matsubayashi, Masahito; Rhodes, N.*; Schoonveld, E.*
JAERI-Research 2004-020, 19 Pages, 2004/12
no abstracts in English
Yamamoto, Kazuyoshi; Kumada, Hiroaki; Kishi, Toshiaki; Torii, Yoshiya; Sakurai, Yoshinori*; Kobayashi, Toru*
Proceedings of 11th World Congress on Neutron Capture Therapy (ISNCT-11) (CD-ROM), 15 Pages, 2004/10
To carry out the boron neutron capture therapy (BNCT) using the epithermal neutron, the epithermal neutron beam intensity was measured by using Au reaction rate activated on the resonance absorption peak (4.9eV). Two scaling factors, which are the reactor power calibration factor and the calculation/experiment (C/E) scaling factor, are necessary in order to correct with the simulation and actual irradiation experiment. First, an optimum detector position was investigated using MCNP code. The result of MCNP calculation showed that the influence of subject placed at the collimator was below 1% when the detector was placed in the distance of over 20cm from the collimator. Therefore we installed the monitor holders near the bismuth block in order to set three gold wire monitors. The factors were determined in the calibration experiments that measure the thermal neutron flux in the phantom and reaction rate of the gold wire monitors. The monitoring technique to measure epithermal neutron beam intensity was applied to clinical irradiation with the epithermal neutron beam.
Endo, Akira; Yamaguchi, Yasuhiro; Sumita, Kenji*
Journal of Nuclear Science and Technology, 40(8), p.628 - 630, 2003/08
Times Cited Count:4 Percentile:31.64(Nuclear Science & Technology)no abstracts in English
Maehira, Takahiro; Hotta, Takashi; Ueda, Kazuo; Hasegawa, Akira*
Journal of the Physical Society of Japan, 72(4), p.854 - 864, 2003/04
Times Cited Count:75 Percentile:90.08(Physics, Multidisciplinary)In order to investigate electronic properties of recently discovered heavy fermion superconductors CeTIn (T=Ir and Co), we employ the relativistic linear augmented-plane-wave (RLAPW) method to clarify the energy band structures and Fermi surfaces of those materials.The obtained energy bands mainly due to the large hybridization between Ce and In 5 states well reproduce the Fermi surfaces consistent with the de Haas-van Alphen experimental results. For the purpose, we construct a tight-binding model for CeTIn by including - and - hoppings as well as - hybridization, which are expressed by the Slater-Koster integrals, determined by the direct comparison with the band-calculation result. Similarity and difference between CeIrIn and CeCoIn are discussed based on the obtained tight-binding model, suggesting a significant importance of the effect of crystalline electric field to understand the difference in electronic properties among CeTIn.
To, Kentaro; Katagiri, Masaki; Sakasai, Kaoru; Matsubayashi, Masahito; Birumachi, Atsushi; Takahashi, Hiroyuki*; Nakazawa, Masaharu*
Nuclear Instruments and Methods in Physics Research A, 485(3), p.571 - 575, 2002/09
Times Cited Count:2 Percentile:18.93(Instruments & Instrumentation)no abstracts in English
Noguchi, Masayasu*; Komine, Takashi*; Kamioki, Hiroshi; Matsumoto, Mikio*
Radioisotopes, 50(7), p.301 - 307, 2001/07
no abstracts in English
; Torii, Yoshiya; ; Ichimura, Shigeju; *; Sasajima, Fumio; *; *; *; Takahashi, Hidetake
JAERI-M 94-058, 45 Pages, 1994/03
no abstracts in English
Amano, Hikaru
Proc. of the 4th Int. Seminor of Liquid Scintillation Analysis, p.185 - 209, 1991/00
no abstracts in English
Ikezoe, Hiroshi; Shikazono, Naomoto; Nagame, Yuichiro; Sugiyama, Yasuharu; Tomita, Yoshiaki; Ideno, K.; Iwamoto, Akira; *
Physical Review C, 42(1), p.342 - 353, 1990/07
Times Cited Count:34 Percentile:85.86(Physics, Nuclear)no abstracts in English
; ; ; ;
Nuclear Physics A, 462, p.150 - 162, 1987/00
Times Cited Count:11 Percentile:55.9(Physics, Nuclear)no abstracts in English